First of all, you must have chosen Bulbasaur for your starter. If not, you can't catch Entei without cheating or hacking. You also must have beaten the Elite Four and have the National Pokédex.
Buy about 20 Max Repels. If you need more later, buy them.
Get a Pokémon at level 49 or very close to that level. You can get a level 49 Pokémon in Cerulean Cave.
Put the level 49 Pokémon in the lead slot. Put on a Max Repel.
Remember, Entei changes its area when you enter a new location, such as changing routes, entering caves, or entering a town. He moves even farther away when you Fly. Entei may move to the route you just entered, with a ton of luck! By the way, you need the Repel and level 49 Pokémon because Entei is level 50. It repels all other Pokémon.
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